A rigorous proof is given for the convergence of the solutions of a viscous Cahn–Hilliard system to the solution of the regularized version of the forward-backward parabolic equation, as the coefficient of the diffusive term goes to 0. Non-homogenous Neumann boundary conditions are handled for the chemical potential and the subdifferential of a possible non-smooth double-well functional is considered in the equation. An error estimate for the difference of solutions is also proved in a suitable norm and with a specified rate of convergence.
In this paper we perform an asymptotic analysis on the viscous Cahn–Hilliard initial-boundary value problem
as , to obtain the regularized diffusion problem in which (1.2) and (1.3) are replaced by the respective equation and condition
Here, Ω is a smooth bounded domain in with boundary Γ and stands for some final time. The variable y denotes some order parameter which may represent the concentration of a phase, and in (1.1)–(1.2) the other variable w plays as chemical potential. The data of the system are the viscosity coefficient , the given functions λ and g in Q, which depend on the space and time positions as well as the boundary datum h on Σ, and the initial value in Ω. Note that the boundary conditions in (1.3) are both of Neumann type, and the one for the chemical potential is preserved in the limit procedure, as in (1.6). Quite unusually for Cahn–Hilliard type problems, this condition is more general that the standard homegeneous one, and this makes that the mean value of y is not conserved in time, as the simple integration on (1.1) on Ω would imply.
The nonlinearities β and π have different properties, although both are equal to 0 in the critical value 0: π is simply Lipschitz continuous, while β represents a continuous increasing function that is allowed in our analysis to become a maximal monotone graph in . Of course, in the case of a multivaled graph β, (1.2) and (1.5) should be properly meant as inclusions (instead of equations), and the assumption on the value of β in 0 must be read as . The point is that, in both situations, β is the subdifferential of a convex and continuous function and, letting , , it turns out that the contribution results from the (sub)differentiation of the following energy functional
Note that, taking for a moment λ constant, the sum
may be seen as a generalization of the well-known double-well potential , actually corresponding to the choices , , . The presence of a coefficient λ varying in space and time is certainly of interest in some cases, for instance you can think to families of control problems in which some linearization has been carried out (cf., e.g., [10–12]).
Let us now comment on the two problems. If we combine (1.1) and (1.5), but without the term , we obtain the nonlinear diffusion equation
which can be derived starting from the mass-balance law
where h denotes the flux of diffusant and is related to the gradient of the chemical potential w according to the Fick law:
The equation of state
contains a nonlinear relation between w and y, via the derivative of the energy function ψ. As ψ is in general the sum of a convex function and a concave perturbation, is non-monotone and the resulting equation (1.7) may be ill-posed.
Then, suitable regularizations are in order, and the most celebrated one is the elliptic regularization
with δ positive coefficient related to surface tension; (1.11) leads to the well-known Cahn–Hilliard system[5,15]. Other choices have been considered in the literature: in particular, Novick–Cohen and Pego[20] dealt with the viscous regularization
which has been recently revisited by Tomassetti [21] (see also the list of references in [21]). In fact, the mathematical problem studied in [21] turns out to be a special case of (1.1), (1.4)–(1.6) and the existence proof in [21] is carried out by working with a Faedo–Galerkin scheme.
The reader can also examine the paper [3] in which a more general non-smooth regularization of the form
γ being a maximal monotone and coercive graph, is considered and the related initial–boundary value problem is investigated when taking Dirichlet boundary conditions for the chemical potential.
On the other hand, a combination of viscous and energetic regularization leads to the so-called viscous Cahn–Hilliard equation (cf. (1.2))
derived by Novick–Cohen[19] and analytically investigated in [13,14], with numerical aspects treated in [1]. Other recent contributions [6,8,10,16,17] deal with Cahn–Hilliard or viscous Cahn–Hilliard equations with singular potentials. Moreover, and this is important for a comparison with our approach, we point out the article [9], in which a wide class of evolution equations, but with monotone nonlinearity, is obtained as asymptotic limit of special Cahn–Hilliard systems. Also, we mention the papers [7,11,12,18,22,23] regarding optimal control problems for some Cahn–Hilliard systems that possibly include dynamic boundary conditions.
In the present contribution, we first recall a precise well-posedness result for the problem (1.1)–(1.4). The statements of other results are also contained in Section 2. Then, in Section 3 we derive a number of estimates, independent of δ, on the solutions to (1.1)–(1.4) and pass to the limit, as δ tends to 0, using properties like compactness, monotonicity and lower semicontinuinity. Thus, we prove the convergence to the solution of (1.1), (1.4)–(1.6) and this convergence proof, in our opinion, deserves some interest since at some points the result cannot be taken for granted. Of course, we have to make assumptions on the data: concerning the maximal monotone graph β in (1.2) and (1.5), we have to require that (see the later (2.16)) the growth at infinity is controlled by the one of the related convex function . But this looks quite reasonable in the framework of (1.5) and less restrictive than the growth of order p assumed in [21]. Actually, by this rigorous asymptotic we give an alterative proof of the existence of solutions to the limit problem (1.1), (1.4)–(1.6). Moreover, for this problem we show the continuous dependence on the data , g, h, and consequently the uniqueness of the solution, in Section 4. Last but not least, strengthening a bit the assumptions on λ and g, we are able to deduce an asymptotic error estimate for the difference of the solutions of the two problems: the proof is given in Section 5.
Main results
In this section, we give some precise formulation of the problems and state our results. Let us first recall the working framework:
Then, Ω is the spatial three-dimensional domain, Γ denotes its boundary, while Q and Σ represent the related spatiotemporal sets. In addition, we adopt the notations
and we will denote the duality pairing between and V with the symbol . As usual, we make the identification , so that H is continuously embedded in in the standard way: for all and , we have , where is the inner product of H.
Secondly, let us recall some useful tools which are often used in dealing with the Cahn-Hilliard equations: the reader can refer to [10, Section 2, pp. 979–980]. We introduce the notation
which specifies the mean value of the elements of , and we recall that
Moreover, we define the operator
by setting as the unique solution with null mean value to the generalized elliptic equation with homogeneous Neumann boundary conditions, i.e.,
Furthermore, if we set as
then is a norm on , equivalent to the usual norm , which makes a Hilbert space. Finally, we recall that
while for all such that for all we have that
Now, it is time make some rigorous assumptions on the data. We assume that
so that is a maximal monotone operator with domain and satisfying the condition . Please notice also that we have .
We are now ready to focus on our problem and present the main results of the paper. As we have anticipated, the aim of the work is to take the limit as in problem (1.1)–(1.4) to show the convergence of the solutions and provide an asymptotic estimate of the error. More specifically, we present now four fundamental results. The first one ensures that problem (1.1)–(1.4) is well posed in a certain variational formulation; the second one is the effective convergence result as and provides the rigorous formulation of the limit problem; the third one is a continuous dependence result for the limit problem and the fourth one contains the asymptotic error estimate.
In the following, we assume to work in the setting (2.1)–(2.4) and (2.13)–(2.14); moreover, we let
and additionally require that
where denotes the minimum-norm element of , for any . We note that, for example, all functions with polynomial and first-order exponential growths comply with our assumption (2.16). In addition, we point out that (2.16) implies (actually, it is equivalent to) the condition
for the same constant C, as checked precisely in the next remark.
Such an equivalence property holds for a more general growth condition and in the general setting of Hilbert spaces. Indeed, let X be a Hilbert space, be convex and l.s.c. (thus continuous since it is everywhere defined), and be a continuous function. If and, for every , is the element of having minimal norm, from the condition
it follows that
Let us check that. If , and , the monotonicity of β implies
Then, by applying (2.18) to , we infer
and letting we recover (2.19) thanks to the continuity of .
Now, we recall a well-posedness result for the problem with . In order to keep a convenient notation henceforth, differently from (1.1)–(1.4) now we put the subscript δ to the solution and denote by the initial value corresponding to δ.
Letand assume thatThen, there existsatisfying for almost allthe variational equalitiesand such thatFurthermore, ifand we letdenote any respective solutions to problem (
2.25
)–(
2.28
) corresponding to the data in (
2.29
)–(
2.30
), then there exists a positive constant C, depending only on τ, the constant in (
2.11
),, a Lipschitz constant for π, Ω, and T, such that
Please note that the equations (2.25)–(2.26) are the natural variational formulations of (1.1) and (1.2), obtained testing by and integrating by parts, on account of the boundary conditions in (1.3).
The proof of Theorem 2.2 is omitted in this work, since the reader can refer to similar results shown in, e.g., [10, Theorems 2.2 and 2.3] and [9] for related details. For the sake of completeness, the key idea is to approximate the problem using the Yosida regularization instead of β and recover a solution of the approximating problem. Then, some uniform estimates are found for this family of solutions and a passage to the limit as provides the solution to the original problem. Let us notice that here the approximation in ε should be carried out with fixed. However, we think that the reader can reconstruct the basic steps of the proofs by examining the estimates (independent of δ) we will prove in Section 3 and compare with Section 4 for the proof of (2.32).
Assume (
2.20
)–(
2.21
) andThen, there exists a familyand a positive constant M such thatFurthermore, for everyletbe the solutions to problem (
2.25
)–(
2.28
) with data. Then, there exists a tripletwhich solves the problemand a subsequence, withas, such that
Theorem 2.4 is the effective convergence result for our problem. Note that the convergence properties (2.44)–(2.47) hold in principle for a subsequence but the next result we state will entail, in particular, the uniqueness of the solution component y. About w and ξ, they are not unique in general but their difference is uniquely determined from (2.41). Then, we can at least claim that the convergence of to y and of to is ensured for the entire family as .
Assume (
2.20
) andLetandbe any respective solutions of the limit problem (
2.40
)–(
2.43
) corresponding to the data in (
2.48
)–(
2.50
). Then, there exists a positive constant C, depending only on τ, the constant in (
2.11
),, a Lipschitz constant for π, Ω, and T, such that
Please note that hypothesis (2.50) is the natural generalization that takes place when dealing with a non-homogeneous Neumann boundary condition. As a matter of fact, in the case of homogeneous Neumann conditions for y, the natural requirement is that and have the same mean value (see for example [8,10]); when a boundary datum is introduced, we need to require also that and have the same mean value on Γ, in order to recover two solutions and with same mean value on Ω at almost every time, so allowing us to prove the continuous dependence result.
Assume thatbesides (
2.33
). Then, there exists a positive constant C such that the following asymptotic estimate holds for all:
The convergence result
In this section, we present the proof of the convergence result contained in Theorem 2.4. In particular, we will firstly check that an approximation on the initial data satisfying (2.34)–(2.35) actually exists; then, we will find some uniform estimates on the solutions and pass to the limit as .
Let us specify some useful notation that we use in the sequel. If we test equation (2.25) by , we deduce that
consequently, in view of (2.28) and the fact that , we deduce that the function belongs to and
Hence, it is natural to introduce
so that
Owing to (2.21) and (2.33) it turns out that
Existence of an approximating family
For every , let us define as the solution to the elliptic problem
It is well known that and it satisfies the variational equation
hence, testing (3.7) by , owing to the Young inequality it is easy to see that
so that the first estimate in (2.35) is satisfied. Moreover, from (3.8) it follows that there exists and a subsequence such that
and letting in (3.7) we reach
since V is dense in H, it turns out that . Furthermore, the identification of the weak limit implies that the entire family weakly converges to in H; finally, from (3.7) we have
so that in H and also condition (2.34) is satisfied.
It remains to check the second estimate of (2.35). For every , let be the Yosida approximation of β: hence, since is Lipschitz continuous, and we can test (3.7) by , obtaining
Hence, thanks to the subdifferential property and the monotonicity of we have
whence (cf., e.g., [2, Thm. 2.2, p. 57])
for all . Taking the limit as in the above inequality, thanks to the Fatou lemma and condition (2.33) we obtain also the second part of (2.35).
The estimate on
We want to find some uniform estimates on : firstly, let us notice that Eq. (3.4) ensures that, for almost every , , so that makes sense. Hence, we can test equation (2.25) by and (2.26) by: summing up the two equations, the second and third integral on the left-hand side cancel thanks to (2.8). Then, we obtain
Recalling (2.7)–(2.8), we note that
while the subdifferential rule for β together with (2.27) leads to
Hence, taking now into account conditions (2.11)–(2.12) and using the assumptions (2.20)–(2.21) and (2.13)–(2.14) on the data, we integrate on and, with the help of the Young inequality, we deduce that
for all and for some Lipschitz constant of π. Now, in view of (3.5) and the continuity of on (ensured by (2.13) and (2.16)) we have
for some constant C independent of . Hence, taking these remarks into account and recalling that converges in by (2.34), we infer that
Then, the Gronwall lemma ensures that
for all ; finally, since , on account of (3.10) and (3.11) we find out that
The estimate on
Let us now prove some uniform estimate on . Observe that, in view of the regularity (2.23), the variational equality (2.26) yields the equation
along with the Neumann homogeneous boundary condition a.e. on Σ. Hence, we can take in (2.25) and test (3.14) at time t by . Note that this makes sense since is in . Summing up the two equations, the second and third integral on the left-hand side cancel thanks to (2.8): hence, using condition (2.10) and integrating on , for almost every we have
As in the previous subsection, using (2.7)–(2.8) we see that
while a well-known result (contained for example in [4, p. 73]) ensures that
hence, using the Young inequality and taking into account conditions (2.11), (2.13)–(2.14), (2.20)–(2.21) and the growth assumption (2.17) (cf. (2.16) and Remark 2.1), we deduce that for almost every
for some constant . Now, thanks to conditions (2.35), (3.10), (3.13) and the Lipschitz continuity of π, we can apply the Gronwall lemma and infer that (updating the value of C, as usual)
for all . Hence, using (3.10) and (3.13) again we conclude that
The estimate on
We now take in Eq. (2.25); by (2.6) we obtain
for almost all and for some two positive constants C and . Then, recalling the estimate (3.17) just proved and hypothesis (2.21) on h, we deduce that
Moreover, taking in (2.26), thanks to (2.16) for almost all we have
so that recalling (3.16), (3.17), and the hypothesis (2.21) on g we infer
and this uniform bound, along with (3.18), ensures that
The estimate on
Next, we would like to show a uniform estimate for in . Let us deduce it on some approximating problem in which β is replaced by its Yosida regularization . Indeed, the estimate, independent of , will be proved for , where denotes the main component of the approximating solution. Then, passing to the limit as , one obtains the same estimate for (cf. Remark 2.3).
Let us rewrite (2.26) in tems of and obtaining
Taking , we have
for almost every . Hence, using the monotonicity of , the hypotheses on g, λ and π together with conditions (3.17) and (3.19), from integration with respect to time and the elementary Young inequality it follows that
for a constant independent of both δ and . Consequently, bearing in mind what we have anticipated before, we conclude that
Let us point out a consequence of (3.20): by a comparison of the terms in (3.14) we deduce that
Moreover, (3.13), (3.21) and well-known elliptic regularity results imply that
The passage to the limit
We are now ready to pass to the limit and conclude the proof of Theorem 2.4. First of all, we notice that the estimates (3.17), (3.19), (3.20), (3.21) ensure that there exist
such that, at least for a subsequence,
as . Moreover, in view of (2.14) and (3.17) there is some such that
We also note that tends to 0 strongly in and weakly in , due to (3.17) and (3.22).
Then, we can pass to the limit in (2.25) to readily recover (2.40) and in (3.14), obtaining (cf. (2.20) too)
From (3.24), using the Ascoli theorem, it follows that
We have to show that
We show the two inclusions together using a unifying argument: the main problem is that the operator is not maximal monotone, so that we cannot rely directly on the lim sup inequality. To this aim, we multiply (3.14) by the test function and integrate over space and time, with to be chosen soon. The idea is that this specific test function induces a linear perturbation (which will be named L) on the operator in the resulting equation, and a smart choice of R gets the sum to be maximal monotone. This will allow us to use some classical tools of monotone analysis to prove the two conditions (3.31) at the same time.
As , it is easy verify that
Hence, from (3.32) we infer that
We now choose R in order that the operator defined by
be strongly monotone and Lipschitz continuous. In fact, we can take , where stands for a Lipschitz constant for π (see (2.14)). Then, it turns out that (see, e.g., [4, Lemme 2.4, p. 34]) the sum of L and of the operator induced by β on (still denoted by β) is maximal monotone. As
is an admissible scalar product in , if we can show that
then, on account of (3.24), (3.27), (3.28) and using a standard result for maximal monotone operators (see, e.g., [4, Prop. 2.5, p. 27]), we actually prove that
In order to check (3.35), we pass to the lim sup in the inequality (3.33) noting that
where the last inequality is a consequence of the weak convergence of to in H for all and of the lower semicontinuity property of the norm in H. Note that the mentioned weak convergence can also be invoked to obtain the initial condition (2.43) from (2.28). Then, using the equality (3.29) tested by , we easily conclude that
whence (3.35) follows.
At this point, we derive the strong convergence
To this aim, we take the difference between (3.14) and (3.29), multiply by the test function and integrate over , with . Taking into account the already performed computations, it is straightforward to verify that
Note that the integral on the second line of (3.38) is non-negative due to the monotonicity of the operator (cf. (3.34) and (2.13)) and to (2.27) and (3.36). Moreover, on account of (2.34), (3.25), (3.26) and (3.30) the right-hand side of (3.38) tends to 0 for all . This implies (3.37) as well as
Then, (2.45) follows from (3.30) and (3.39); moreover, the Lipschitz continuity of π enables us to conclude that strongly in , whence from (3.28). At this point, it is not difficult to deduce (3.31), and in particular (2.42), from (3.36), as
Hence, Theorem 2.4 is completely proved. As a further remark, we note that the boundedness of in and the convergence (3.37) (or the first one in (3.39)) ensure that strongly in for all .
Continuous dependence for the limit problem
This section is devoted to proving the continuous dependence result for the limit problem. Assume thus the hypotheses of Theorem 2.6 and let , , be any respective solutions corresponding to the data in (2.48). For simplicity, let us introduce the notation
Hence, if we subtract the corresponding equations (2.40)–(2.41), for almost every we have
Please note that hypothesis (2.50) ensure that , so that we test (4.1) by and (4.2) by : summing up, the second and third integral on the left-hand side cancel thanks to (2.8). Therefore, for almost every we infer that
Then, in view of (2.10)–(2.12) and the monotonicity of β, integrating on leads to
for a.e. and a certain constant . Now, we can apply the Gronwall lemma that implies (updating the value of C)
and the estimate (2.51) is proved.
Asymptotic error estimate
In this section, we prove the asymptotic estimate stated in Theorem 2.8. To this aim, in a first step we deduce an additional uniform estimate to improve the boundedness properties of the solution to the problem (2.25)–(2.28).
The estimate on
Here, we want to prove something better than (3.21). We test (3.14) by and deduce that
for almost all . Please note that the second term on the left-hand side can be written by integration by parts as
let us handle the terms on the right-hand side. We integrate by parts, taking into account that satisfies Neumann homogeneous boundary conditions. By the Young inequality we have
moreover, proceeding formally as we already did in Section 3.5, it is not restrictive to argue with instead of , so that using monotonicity we deduce that
Finally, using the hypotheses on λ and π and the Young inequality, a direct computation leads to
Hence, taking all these remarks into account, integrating (5.1) with respect to time, and using (3.17), (3.19) and the hypotheses (2.20)–(2.21) we obtain
for some constant ; then, using the Gronwall lemma and condition (2.35), we conclude that
Error estimate
In order to prove Theorem 2.8, we subtract (2.25) and (2.26) to (2.40) and (2.41), respectively, and for almost every we have
Testing the first equation by and the second by , we sum up with the help of (2.8) to cancel the two integrals on the left hand side, as usual. Hence, integrating by parts we obtain for almost every
now, the monotonicity of β, the hypotheses (2.14) and (2.20), and the Young inequality lead to
so that the Gronwall lemma and the estimate (5.2) allow us to infer that
for a certain constant . This finishes the proof. Let us point out that the error estimate (2.54) is of order in terms of δ provided : this condition is ensured for the family defined in (3.6) whenever, for instance, (take in (3.7) and perform the estimate).
Footnotes
Acknowledgements
The first author gratefully acknowledges some financial support from the GNAMPA (Gruppo Nazionale per l’Analisi Matematica, la Probabilità e le loro Applicazioni) of INdAM (Istituto Nazionale di Alta Matematica) and the IMATI – C.N.R. Pavia.
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