Based on previous homogenization results for imperfect transmission problems in two-component domains with periodic microstructure, we derive quantitative estimates for the difference between the microscopic and macroscopic solution. This difference is of order , where describes the periodicity of the microstructure and depends on the transmission condition at the interface between the two components. The corrector estimates are proved without assuming additional regularity for the local correctors using the periodic unfolding method.
This paper considers a class of linear elliptic equations with an imperfect transmission condition modeling, for instance, heat conduction, diffusion, or stationary current flow in a composite material. The macroscopic domain Ω consists of a connected component and a second component , which is the collection of periodically distributed inclusions or pores. The characteristic length scale of the microstructure, given by the distance between two such pores, is of order ε. On the interface between the two components, the flux is proportional to the jump of the solution across this interface, which models e.g. a contact resistance. The corresponding proportionality factor is of order with . More precisely, we consider for the problem
where is the unit outer normal to for . The matrix and the coefficient are ε-periodic and uniformly bounded. Moreover, we suppose that is uniformly elliptic, is strictly positive, and the source term f is square-integrable.
For ε tending to zero, the homogenization limit of problem (1.1) has already been well studied in the literature. Based on Tartar’s method for oscillating test functions, the homogenization limit was derived for all in [11,26]; see references therein for earlier works. This problem was also treated for two connected components [3], poly crystals [21], for stochastic microstructures [20], and evolution problems [8,22]. Recently, the homogenization limit and strong two-scale convergence of the gradients were proved in [10] for via the method of periodic unfolding. However, up to now all publications contain qualitative results, whereas, this paper provides quantitative corrector estimates.
In the limit , we obtain one homogenized elliptic equation posed in the whole macroscopic domain
The constant matrix depends on γ, whereby we distinguish the following three cases: (i) for , (ii) for , and (iii) for . The case is not treated here, since it allows for unbounded solutions as it is shown in [21].
For , the jump across the interface is negligibly small such that is given via the standard unit cell problem on the whole reference cell, see (6.2) for more details. In other words, the model in (1.1) behaves for like a classical Poisson equation with ε-periodic coefficients in a one-component domain.
For , the matrix is obtained by solving a unit cell problem in two sub-domains of the reference cell separated by an interface, see (5.2). In this case, the unit cell problem reflects the structure of (1.1) on the level of the reference cell and the effective matrix takes the imperfect transmission condition into account. Indeed, this is the only case, where the effective matrix depends on the values of the boundary term .
For , we obtain the same effective matrix as in [7], cf. (4.2), wherein the homogenization of the Poisson equation is considered in the perforated domain with no-flux boundary conditions at the holes. In their situation, the function f is multiplied by the ratio of the volume of the occupied domain divided by the total volume of Ω. However, this ratio does not appear in (1.2) which shows that the exchange between the two components is sufficient in order to take into account also the source term in .
The main result of this paper are the quantitative error estimates between the microscopic solution , the macroscopic limit u, and their corresponding correctors for the three different cases: (i) in the Theorems 4.1 and 4.3, (ii) in Theorem 5.1, and (iii) in Theorem 6.3. In the special case , the jump across the interface is of order and it depends on , and the volume fraction of the component . To prove this result in Theorem 4.3, we require additional -regularity for the source term f and that is constant. In the case , Lipschitz continuity of the matrix is assumed for technical reasons.
For all , the -corrector estimates are of order with , and in the special cases or we recover the maximal convergence rate . In order to prove these quantitative estimates, we need that the limit u is of higher -regularity, whereas and as well as the local correctors are in general only -regular. The derivation of the corrector estimates relies on the two-scale formulation of the limit (1.2) as in [10], the periodic unfolding method as in [4,5], and unfolding based error estimates as in [15,16,28]. The key step of the proofs is to construct the correct approximating sequences via defining suitable recovery operators. Those operators recover the oscillations of the gradients in the components and from the macroscopic limit and the local correctors. Especially for the case (i), the new operator is introduced in (3.6) in order to capture the “flatness” of the gradient within the inclusions.
The text is structured as follows. In Section 2, we present the model as well as all necessary assumptions and notations. In Section 3, the periodic unfolding method is introduced and we define the unfolding and folding (averaging) operator and, in particular, the recovery operators in Section 3.1. In the case (i), the corrector estimates are given in Section 4. Therein, we distinguish the cases (Theorem 4.1) and (Theorem 4.3) in the Sections 4.1 and 4.2, respectively, although they share the same effective matrix. The remaining corrector estimates for the cases (ii) and (iii) are given in the Sections 5, and 6, respectively. We conclude the presentation with a brief discussion in Section 7 and a possible application to supercapacitors in Section 7.1.
The two-component domain Ω (left) and the reference cell Y (right).
The imperfect transmission problem posed in a two-component domain
Throughout the text we postulate the following assumptions on the domain and the periodic microstructure as shown in Fig. 1.
The macroscopic domain Ω is a d-dimensional polytope with , i.e. it is
The reference cell is the disjoint union of the subsets and , where is open, connected, and satisfies . The inner boundary is Lipschitz continuous and it holds .
Let denote the set of nodal points inside Ω. The two disjoint components and , and their common boundary are given via
The microscopic period is given via with such that Ω is the exact union of translated cells with for all ε.
By construction, the set is connected, bounded, and has a Lipschitz boundary, whereas the set consists of isolated inclusions. The former implies the existence of extension operators mapping from to , where the subscript D indicates homogeneous Dirichlet boundary conditions. Indeed, is the disjoint union of and , and it is
The assumption that does not touch the boundary of the reference cell Y is essential for the construction of the recovery operator in (3.6), see Remark 3.1. This assumption is also contained in [10].
The Assumption (D4) significantly simplifies the presentation of the corrector estimates, however, the results remain valid for arbitrary domains Ω with smooth boundary and . In such a case, one considers bigger domains , , satisfying again (D2)–(D4) and uses Lemma A.6 to control the error at the boundary (cf. [15,16,28]). In any case, we have to avoid cells intersecting the boundary such that is always a Lipschitz domain (cf. also [10, Fig. 2]).
In order to obtain unique and bounded solutions for the microscopic respective homogenized problem, we require the following assumptions for the given data. The dot “” always denotes the scalar product in .
The matrix is Y-periodic, symmetric, and uniformly elliptic, i.e.
The boundary term h is a Y-periodic function in and satisfies
It is and the coefficients of the microscopic problem are given via
Under the above assumptions, the Lax–Milgram theorem yields the existence of a unique solution for the weak formulation of the microscopic problem (1.1) (cf. [26, Section 1]), i.e. find such that
for all admissible test functions . Moreover, this solution satisfies the following a priori bounds.
Any solution of the microscopic problem (
1.1
) is bounded for allviawhere the constantis independent of ε.
The solution of the homogenized problem (1.2) is unique and bounded, too. Moreover, u is of higher regularity, since the macroscopic domain Ω is a bounded convex polytope. Indeed, it holds according to [18, Thm. 3.2.1.3]
where only depends on the effective matrix and the domain Ω. The precise definition of depends on the three different regimes (i)–(iii) for γ and it is given in the corresponding section.
Periodic unfolding
Following [4 ,6,10], we define the periodic unfolding operators and , which map one-scale functions on the oscillating domains and to two-scale functions on the fixed domains and , respectively. Therefore, let denote the standard two-scale decomposition of every into its integer part and the remainder . For any Lebesgue measurable function u on the periodic unfolding operator is given via
and it satisfies the integration formula
Within the inclusions, we define for any Lebesgue measurable function u on the second periodic unfolding operator by (cf. [10, Def. 2.8])
In particular, both periodic unfolding operators are well-defined for functions u on Ω via the relation , for , with denoting the characteristic function of the set . Moreover, the restriction of to Lebesgue measurable functions u on is also well-defined and it is almost everywhere in . We recall that for Sobolev functions the unfolding belongs to the space , for all and . Then, if the traces of and coincide in , so do the traces of and in . There holds the following integration formula for boundary unfolding (cf. [6, Prop. 5.2])
We complete this collection by introducing the folding operator (sometimes called averaging operator) 1
Note that and can be identified for , whereas this fails for .
for and via
where denotes the usual average over the domain . Here, and in the following, denotes the d-dimensional Lebesgue measure of domains respective the -dimensional Lebesgue measure of hypersurfaces.
According to [4,10], the folding operator is the adjoint of , i.e.
In the same manner, is the adjoint of . Finally, we note that the periodic unfolding respective averaging operator, and , as introduced in [5] are given via
Construction of recovery operators
In this section we introduce two operators, and , which will help us to construct suitable recovery respective approximating sequences for the derivation of the corrector estimates. To do so, we define the scale-splitting operator following [5, Def. 4.1]. Let denote the extension of according to [27, Thm. 3.9]. For and every , we set
and
The function interpolates the values of at the nodes via -Lagrange elements as customary in the finite elements methods. Since is (weakly) differentiable, in contrast to , we can use the scale-splitting operator to construct oscillating one-scale functions that recover global corrector-type functions . Let respective denote the space of Y-periodic Sobolev functions, i.e.
For any Y-periodic function, we may identify with for all .
For and , the approximating sequence is given via (cf. [15])
The cut-off function satisfies for all with and ; and it guarantees the Dirichlet boundary condition on . We may also call recovery respective gradient folding operator, since it holds and in . The uniform boundedness of the scale-splitting operator according to [5, Prop. 4.5] implies the following bound
On the perforated domain , we adjust the construction of the approximating sequence as follows: for , the sequence is given via
In the same manner, we define for the sequence via
Notice that is skipped in (3.5), since the inclusions is not equipped with Dirichlet boundary conditions. Here, we also use , since is in general not Y-periodic.
We introduce the second recovery operator in the inclusions as follows: define
and observe that the gradient is constant with respect to all . Recall that for every , the two-scale decomposition gives with and . With this, the recovery operator , given via
is well-defined and it holds . Moreover, we recover the convergences and in .
We point out that is in general not Y-periodic. However, since it holds , we can periodically extend to and, by translation, also to the whole space . With this, we may also construct on the whole domain Ω. Notice that this construction fails in the case .
Otherwise, if and are connected for , there also exists a suitable extension operator and we may treat in a similar manner as .
Corrector estimates for
We begin with recalling the two-scale convergence of the solutions of the microscopic problem (1.1) as it is shown in [10, Sections 3.2 & 4.3]. There exist limit functions and with such that
Moreover, we distinguish the following two cases
where . The quantity characterizes the jump across the interface . In the limit , the pair solves the weak two-scale formulation
for all and . The macroscopic function u is in particular the solution of the homogenized equation (1.2), wherein the effective matrix is constant and it is given for all via the formula
Here, denotes the canonical basis of and are the local correctors. The latter are the solutions of the cell problem for
where denotes the unit outer normal to . We point out that the effective matrix and the local correctors only depend on the values of restricted to the subset . In other words, the values of and do not enter the limit problem, as if the second component contained only “empty space” in the first place. The corresponding global corrector is given via the formula
Note that the higher regularity of the limit solution implies also the higher x-regularity of the global corrector .
The case
Let the assumptions (D1)–(D4) on the microstructure and (A1)–(A3) on the data hold true. Then, the solutionsand u of the microscopic problem (
1.1
) and the homogenized equation (
1.2
), respectively, satisfy forwhere C is a positive constant independent of ε.
The derivation of the estimates follows the principle idea of the unfolding based estimates in [15,16]. In particular the control of the periodicity defect of , which is in general not Y-periodic for arbitrary functions , is proved in these two articles.
By assumption it holds .
Step 1: Periodicity defect. In the weak formulation (4.1), we choose the two-scale test function according to Theorem A.3 such that it holds
where only depends on Ω and . Exploiting this estimate with the higher x-regularity of 2
Notice that the spaces and can be identified.
as well as the duality of periodic unfolding operator and folding operator yields with
Using , the definition of in (3.4), the boundedness of the linear operator from into itself, the assumptions and , as well as the Lemmas A.1, A.5, and A.6 give
where denotes the ε-neighborhood of the boundary . We finish Step 1 with
Step 2: Admissible test functions. We test the weak formulation of the microscopic problem (2.1) with
and arrive at
According to Theorem A.7, the extension satisfying is an admissible test function for the limit problem in (4.4). Subtracting (4.6) from the left-hand side in estimate (4.4) and recalling gives
With Young’s inequality and to be specified later, it holds
Step 3: Approximation errors. Inserting into (4.7), we estimate the boundary term of lower order with and (A.2) via
The source term on the right-hand side of (4.7) is estimated with (A.1) and
Recalling that , we control the -term in (4.7) via
Here, we used that for all (with denoting the Hessian) according to (3.6) and, hence, it is
Combining the error estimates in (4.9)–(4.11) with (4.7)–(4.8) gives
Exploiting that is uniformly elliptic and , choosing and , as well as applying Poincaré–Friedrich’s inequality to yields
The desired estimate (4.3) follows by taking the square root. □
To see that the -estimate in (4.3) is analogous to the -estimate in [15, Prop. 4.3], we can control the term by as in Step 1 and obtain
The case
In order to characterize the jump across the interface , we impose two additional assumptions on the given data, i.e.
With this, we simply have for all as well as . The extra regularity for the source term f is needed to apply the recovery operator and concerning h’s regularity we refer to Remark 4.4.
Let the assumptions of Theorem
4.1
as well as in (
4.13
) hold true. Then, there exists a positive constant C independent of ε such that it holds
Step 1 of the proof is exactly as in the case and in what follows we only outline the modifications in Steps 2 and 3.
Step 2: Admissible test functions. For the weak formulation of the microscopic problem, we choose the test functions as in (4.5) and
Thus, we arrive at
Step 3: Approximation errors. Inserting into (4.15), we obtain for the boundary term
The absolute value of the third term (on the right-hand side) above is bounded by as in (4.9). For the source term in (4.15), we obtain
and again the absolute value of the second integral is bounded by . It remains to control the following difference using the integration formula (3.2)
where denotes the indicator function of the set . Recall that the traces of and coincide on and, hence, it holds almost everywhere in . After suitably rearranging the integrands, we get
Here, Lemma A.2 yields the -estimate for f and belonging to the space . Moreover, the integral term in (4.16) vanishes as follows: the function is constant with respect to x in each microscopic cell and it holds
as well as with
Since the difference (4.17) − (4.18) vanishes on each subset and Ω is the exact union of translated cells, the whole integral vanishes in (4.16). Treating the gradient terms in (4.15) as in (4.8) and (4.11), we overall arrive at
which gives estimate (4.14). □
The extra assumption on the boundary function stems from the fact that the following equality only holds true for constant functions h
This identity is needed for the equality of (4.17) and (4.18). So far, the only generalization for functions are small perturbations of order ε, i.e. .
Corrector estimates for
This case is in some sense more special than (i) and (iii), since the limit problem depends indeed on all values of in the whole reference cell Y and the boundary term . So, we recover on the level of the reference cell again an imperfect transmission problem, see (5.2). According to [10, Sections 3.4 & 4.2], there exist three limit functions as well as and with such that
Moreover, the triple solves the weak two-scale formulation
for , , and . The macroscopic function u solves indeed the homogenized equation (1.2) and the effective matrix is given via
Here, and solve the following cell problem for
where and denote the unit outer normal to and , respectively. Thanks to the higher regularity of the limit u, the corresponding global correctors and belong to the spaces and , respectively. They are given via
Let the assumptions of Theorem
4.1
hold true. Then, there exists a positive constant C independent of ε such that it holds
Step 1: Periodicity defect. In the weak formulation (5.1), we want to choose the two-scale test functions
with arbitrary , however, does not respect the Y-periodicity in general. Compensating the periodicity defect with according to Theorem A.3 and Remark A.4(b) as well as using the duality of and respective and gives
For the boundary term, we also used the continuous embedding of into such that it holds for and ,3
Here, we also used the continuous embedding of into and, hence, .
with as in Remark A.4(b),
Next, we want to replace with (recall (3.5) for ) in the boundary integral in (5.4) via the Lemmas A.1 and A.5. Together with the integration formula (3.1) as well as , we get
The same estimate holds for . Applying the integration formula (3.2) and treating the gradient terms as in the case gives
In particular, the integration formula (3.2) implies , cf. also [10, Eq. (2.8)].
Step 2: Admissible test functions. We test the weak formulation (2.1) with
and choose in (5.5) such that the difference between microscopic and reformulated macroscopic weak formulations reads
Estimating the -integral on the right-hand side as in (4.10), exploiting the uniform ellipticity of and , as well as choosing and suitably gives the desired estimate (5.3). □
Corrector estimates for
In this regime, we recover in the limit the standard unit cell problem. Indeed, there exist according to [10, Sections 3.3 & 4.1] two limit functions and with such that the microscopic solutions satisfy
In particular, the pair is the unique weak solution of the two-scale limit problem
for all and . Moreover, u solves the macroscopic equation (1.2), and the effective matrix as well as the global corrector are given via
where the local correctors solve the standard cell problem for
We aim to derive the corrector estimates in the case in two steps. First, we introduce the standard homogenization problem in the whole domain without any interfaces, so to speak the perfect transmission problem: find such that
for all admissible test functions . This classical problem is well-studied in the literature, and there exist error estimates for the difference of the microscopic solution and the macroscopic solution u of (1.2).
Let the assumptions of Theorem
4.1
hold true. Then, there exists a positive constant C independent of ε such that it holds
In the second step, we control the difference of the solution of the standard homogenization problem and the solution of the imperfect transmission problem. In order to prove such error estimates, we require the extra regularity such that the -norm of can be controlled.
Let the assumptions of Theorem
4.1
as well ashold true. Then, there exists a positive constant C independent of ε such that it holds
In the weak formulations (6.3) and (2.1), we choose the admissible test functions as well as and , respectively. Taking the difference of both formulations gives
Adding under the -integral and using partial integration yields
While noting that in , the two -integrals containing the difference cancel each other. It remains to control the additional boundary term. Applying Hölder’s and Young’s inequality with gives
With estimate (A.2), we arrive at
The additional regularity implies the higher regularity of the solution . Revisiting the proofs of the Theorems 3.1.3.3 and 3.2.1.3 in [18] yields the existence of a constant only depending on the properties of the domain Ω and the ellipticity constant α such that
Using , for , gives , which in turn yields . Inserting the latter into (6.4), yields overall
Finally, choosing as well as exploiting the uniform ellipticity of and gives the desired error estimate. □
Combining the results of Proposition 6.1 and Theorem 6.2 gives immediately the main result of this Section.
Let the assumptions of Theorem
6.2
hold true. Then, there exists a positive constant C independent of ε such that it holds for
The Lipschitz continuity of is indeed a quite restrictive assumption and we expect that it can be generalized in some sense.
(a) Indeed, the difference belongs to the better space and one could study the dual paring
instead of the -scalar product in (6.4). Unfortunately, the -norm of is only of order , which can been seen from . The same problem also occurs when comparing the two solutions and u directly.
(b) There arises the question whether one can construct for any sequence , which is uniformly bounded in and satisfies , a sequence of extensions with and . If this were possible, one could choose more clever test functions in the proof of Theorem 6.2 and would obtain the estimate (only assuming bounded).
Discussion
The present corrector estimates do not require any additional regularity of the microscopic solution or the local correctors. However, we need that the limit satisfies , which is immediate for convex Lipschitz domains or domains whose boundary is of class . In the case , the more restrictive assumptions and h is constant are necessary in order to characterize the jump across the interface. It remains open whether these assumptions can be relaxed. Anyways, the source term has to be more regular than in all the other cases, since we need for all in estimate (4.14). In the third case , we had to impose the Lipschitz continuity of to control the fluxes across the interface. It is to expect that this assumption can be relaxed to discontinuous , however, the proof remains open.
We point out that our corrector estimates recover the convergence rate , in the special cases and . This rate seems to be optimal for corrector estimates up to the boundary of the macroscopic domain as it was also obtained in [15,28] for elliptic equations with periodically oscillating coefficients and without interfaces.
In order to treat double porosity models, which include degenerating terms such as as in [2,12], we can introduce another gradient folding operator. For , the one-scale function is given via the solution of the elliptic problem (cf. [19,25])
In [28 ,29] the folding mismatch between the averaging operator and the gradient folding operator is quantified.
We believe that the imperfect transmission problem can also be considered with non-homogeneous Dirichlet boundary conditions, as it is done in the paper [17] on error estimates with boundary data in .
It is an open problem whether similar corrector estimates can also be proved for nonlinear transmission conditions as in [9,24]. However, we expect that the present results carry over to systems of coupled semilinear parabolic equations with linear transmission conditions. Previously, unfolding-based estimates for reaction-diffusion systems were proved in [14,29].
Application to supercapacitors
A prospective application of models containing imperfect transmission conditions is the supercapacitor, which is a small electrochemical device to store energy. The high capacity of the device is obtained by maximizing the surface area to volume ratio, which is achieved by taking a porous electrode, see Fig. 2.
Let us study the stationary current flow in such a device. First of all we note that discontinuities of the potential are in principle nonphysical. However, when considering a double-layer4
The double-layer is given via the δ-neighborhood of the interface as sketched in Fig. 2.
, where the thickness of the layer δ is much smaller than the pore size ε, we can reduce the double-layer model to an interface model: In [13], the asymptotic limit was studied for one single electrode and one obtains that the normal of the electric displacement across the interface is equal to the surface charge density in one single layer,5
The surface charge density is the line integral of the charge density .
i.e. . Hereby, depends on the relative permittivity , the vacuum permittivity , and the electric field E, where is given via the electrostatic potential φ. Using a linearization argument, we obtain that is proportional to the difference of the electric potential, i.e. , where the proportionality factor C denotes the capacity per surface element.6
The relation between current flux and potential difference is in general not linear, since the capacity depends nonlinearly on the electric potential, see e.g. [23].
Thus, we obtain the interface condition on . Realizing that the total capacity of each electrode is proportional to the ratio of its surface area A divided by the distance between two electrodes yields as in the case (ii). For Carbon-based electrodes, characteristic pore sizes are nanometers, see e.g. [30], and the macroscopic length scale of the device is about several hundreds micrometers. Hence, the parameter ε is of order –.
The main components of a supercapacitor (left) and the double layer (right).
Footnotes
Acknowledgements
The author thanks C. Guhlke, M. Landstorfer, and D. Peschka for helpful discussions on possible applications in Section . Moreover, the author thanks M. Gahn as well as the anonymous referee for their suggestions, which improved the quality of the text a lot. The research of S.R. was supported by Deutsche Forschungsgesellschaft within Collaborative Research Center 910: Control of self-organizing nonlinear systems: Theoretical methods and concepts of application via the project A5: Pattern formation in systems with multiple scales.
Auxiliary estimates
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